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Scott, K.; Kisiel, E.; Yakhou, F.; Agrestini, S.; Garcia-Fernandez, M.; Kummer, K.; Choi, J.; Zhong, R_D; Schneeloch, J_A; Gu, G_D; et al (, Physical Review B)
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Nag, A.; Nocera, A.; Agrestini, S.; Garcia-Fernandez, M.; Walters, A. C.; Cheong, Sang-Wook; Johnston, S.; Zhou, Ke-Jin (, Nature Communications)Abstract The microscopic origins of emergent behaviours in condensed matter systems are encoded in their excitations. In ordinary magnetic materials, single spin-flips give rise to collective dipolar magnetic excitations called magnons. Likewise, multiple spin-flips can give rise to multipolar magnetic excitations in magnetic materials with spin S ≥ 1. Unfortunately, since most experimental probes are governed by dipolar selection rules, collective multipolar excitations have generally remained elusive. For instance, only dipolar magnetic excitations have been observed in isotropic S = 1 Haldane spin systems. Here, we unveil a hidden quadrupolar constituent of the spin dynamics in antiferromagnetic S = 1 Haldane chain material Y 2 BaNiO 5 using Ni L 3 -edge resonant inelastic x-ray scattering. Our results demonstrate that pure quadrupolar magnetic excitations can be probed without direct interactions with dipolar excitations or anisotropic perturbations. Originating from on-site double spin-flip processes, the quadrupolar magnetic excitations in Y 2 BaNiO 5 show a remarkable dual nature of collective dispersion. While one component propagates as non-interacting entities, the other behaves as a bound quadrupolar magnetic wave. This result highlights the rich and largely unexplored physics of higher-order magnetic excitations.more » « less
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Rossi, M.; Lu, H.; Lee, K.; Goodge, B_H; Choi, J.; Osada, M.; Lee, Y.; Li, D.; Wang, B_Y; Jost, D.; et al (, Physical Review B)
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